We are excited to announce that the preprint of our manuscript “Robust Computation and Analysis of Vibrational Spectra of Layered Framework Materials Including Host-Guest Interactions” is now available on ChemRxiv https://doi.org/10.26434/chemrxiv-2024-x8vt1! In this study, we devise robust computational settings for the AIMD-based vibrational spectra of COF-1, and we present a strategy to dissect and analyze the spectra, facilitating the monitoring of particular bands.